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PHYSICAL REVIEW C VOLUME 37, NUMBER 5 MAY 1988 One-nucleon stripping reactions to discrete levels intiuceti by a 480 MeV ' C beam on a 'Pb target M. C. Mermaz, E. Tomasi-Gustafsson, B. Berthier, R. Lucas, J. Gastebois, A. Gillibert, and A. Miczaika Departement de Physique Nucleaire, Centre d'Etude Nucleaire de Saclay, 91191 Gif sur Y-vet-te Cedex, France A. Boucenna, L. Kraus, I. Linck, B. Lott, R. Rebmeister, N. Schulz, and J. C. Sens Centre de Recherche Nucleaire et Uni Uersite Louis Pasteur, 67037 Strasbourg, Cedex, France C. Grunberg Grand Accelerateur National d'Ions Lourds, Caen, 14021 Caen Cedex, France (Received 21 October 1987) One-proton and one-neutron stripping reactions induced by a 480 MeV "C beam bombarding a 'Pb target have been studied using a high resolution energy loss magnetic spectrometer. The reac- tions are governed by two selection rules which are naturally contained in the one-step exact finite range distorted wave Born approximation formalism. Relative intensities of the populated states are well reproduced by this formalism as well as the absolute values of the cross sections. Compar- isons with the results of one-nucleon stripping reactions induced by a ' 0 beam on a ' 'Pb target at 793 MeV incident energy are also presented; in this latter case the absolute cross section values are not reproduced. I. INTRODUCTION One-nucleon transfer reactions have already been ex- tensively studied experimentally and rather successfully compared with the exact finite range-distorted wave Born approximation (EFR-DWBA) predictions. ' We shall present in this paper experimental data and theoretical analyses concerning very high incident energy: one- proton and one-neutron direct surface transfer reactions induced by a 480 MeV ' C beam on a Pb target. These present results will also be compared to our previous data obtained with a 793 MeV ' 0 beam bombarding a 2o Pb target, and already partially published Refs. 4 and 5. At high incident energy the values of the cross sections are governed by two selection rules contained in the EFR-DWBA and also in the semiclassical model of Brink. ' The first selection rule tells us that final states with high spin are strongly favored at high incident ener- gy. This is due to the large mismatch between the en- trance and exit grazing wave orbital angular momenta. The second selection rule tells us that the favored transi- tion involves no spin-flip between the projectile wave function and the heavy residual nucleus wave function. We shall see that these two selection rules explain per- fectly the relative intensities for the population of the single-particle states. ' However, we shall also see that the absolute values are well reproduced by the EFR- DWBA calculations in case of ' C induced reactions, but definitively not in the case of ' 0 induced reactions: a rather puzzling problem. A detailed study of the EFR- DWBA calculations at high incident energy will be presented, and, in addition, the transition to high spin states at higher excitation energy will be tentatively ana- lyzed. II. EXPERIMENTAL ARRANGEMENT The one-proton and one-neutron transfer reactions on a Pb target were performed at the GANIL facility us- ing the 480 MeV ' C beam. The ejectile particles, "B and "C nuclei, were identified and momentum analyzed using the energy loss magnetic spectrometer SPEG (Ref. 8). The thickness of the Pb target (99% enriched) was about 1. 7 mg/cm measured with the alpha gage tech- niques. The detection system consisted of (i) two position (x,y) drift chambers having a spatial resolution of 0. 6 mm in each direction, located on each side of the focal surface in order to determine the scattering angle and the accurate magnetic rigidity of the detected particle, (ii) an ionization chamber which measured the energy loss of the outgoing particles, necessary for their identification, (iii) two plastic scintillators, the first one providing the start signal of the time of flight and the second one serv- ing as a veto for the rejection of light particles. The rf of the last GANIL cyclotron provided the stop signal of the time of flight. All the gas counters were filled with isobu- tane. With this arrangement the measured energy resolu- tion was about 200 keV fu11 width at half maximum (FWHM), or translated into momentum resolution: hp jp =2X 10 . The total angular aperture of the spec- trometer in the reaction plane was 4 and the counting rate normalization between runs was assured by a one de- gree overlap in angle. The beam emittance for all runs was never larger than 2m mm mrad which permits an an- 37 1942 1988 The American Physical Society

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PHYSICAL REVIEW C VOLUME 37, NUMBER 5 MAY 1988

One-nucleon stripping reactions to discrete levels intiuceti

by a 480 MeV ' C beam on a 'Pb target

M. C. Mermaz, E. Tomasi-Gustafsson, B. Berthier, R. Lucas, J. Gastebois,A. Gillibert, and A. Miczaika

Departement de Physique Nucleaire, Centre d'Etude Nucleaire de Saclay,91191Gif sur Y-vet-te Cedex, France

A. Boucenna, L. Kraus, I. Linck, B. Lott, R. Rebmeister, N. Schulz, and J. C. SensCentre de Recherche Nucleaire et Uni Uersite Louis Pasteur, 67037 Strasbourg, Cedex, France

C. GrunbergGrand Accelerateur National d'Ions Lourds, Caen, 14021 Caen Cedex, France

(Received 21 October 1987)

One-proton and one-neutron stripping reactions induced by a 480 MeV "C beam bombarding a'Pb target have been studied using a high resolution energy loss magnetic spectrometer. The reac-

tions are governed by two selection rules which are naturally contained in the one-step exact finite

range distorted wave Born approximation formalism. Relative intensities of the populated states

are well reproduced by this formalism as well as the absolute values of the cross sections. Compar-

isons with the results of one-nucleon stripping reactions induced by a ' 0 beam on a ' 'Pb target at793 MeV incident energy are also presented; in this latter case the absolute cross section values are

not reproduced.

I. INTRODUCTION

One-nucleon transfer reactions have already been ex-tensively studied experimentally and rather successfullycompared with the exact finite range-distorted wave Bornapproximation (EFR-DWBA) predictions. ' We shallpresent in this paper experimental data and theoreticalanalyses concerning very high incident energy: one-proton and one-neutron direct surface transfer reactionsinduced by a 480 MeV ' C beam on a Pb target. Thesepresent results will also be compared to our previous dataobtained with a 793 MeV ' 0 beam bombarding a 2o Pbtarget, and already partially published Refs. 4 and 5.

At high incident energy the values of the cross sectionsare governed by two selection rules contained in theEFR-DWBA and also in the semiclassical model ofBrink. ' The first selection rule tells us that final stateswith high spin are strongly favored at high incident ener-

gy. This is due to the large mismatch between the en-trance and exit grazing wave orbital angular momenta.The second selection rule tells us that the favored transi-tion involves no spin-flip between the projectile wavefunction and the heavy residual nucleus wave function.We shall see that these two selection rules explain per-fectly the relative intensities for the population of thesingle-particle states. ' However, we shall also see thatthe absolute values are well reproduced by the EFR-DWBA calculations in case of ' C induced reactions, butdefinitively not in the case of ' 0 induced reactions: arather puzzling problem. A detailed study of the EFR-DWBA calculations at high incident energy will bepresented, and, in addition, the transition to high spin

states at higher excitation energy will be tentatively ana-lyzed.

II. EXPERIMENTAL ARRANGEMENT

The one-proton and one-neutron transfer reactions ona Pb target were performed at the GANIL facility us-

ing the 480 MeV ' C beam. The ejectile particles, "Band "C nuclei, were identified and momentum analyzedusing the energy loss magnetic spectrometer SPEG (Ref.8). The thickness of the Pb target (99% enriched) wasabout 1.7 mg/cm measured with the alpha gage tech-niques. The detection system consisted of (i) two position(x,y) drift chambers having a spatial resolution of 0.6mm in each direction, located on each side of the focalsurface in order to determine the scattering angle and theaccurate magnetic rigidity of the detected particle, (ii) anionization chamber which measured the energy loss ofthe outgoing particles, necessary for their identification,(iii) two plastic scintillators, the first one providing thestart signal of the time of flight and the second one serv-ing as a veto for the rejection of light particles. The rf ofthe last GANIL cyclotron provided the stop signal of thetime of flight. All the gas counters were filled with isobu-tane. With this arrangement the measured energy resolu-tion was about 200 keV fu11 width at half maximum(FWHM), or translated into momentum resolution:hp jp =2X 10 . The total angular aperture of the spec-trometer in the reaction plane was 4 and the countingrate normalization between runs was assured by a one de-gree overlap in angle. The beam emittance for all runswas never larger than 2m mm mrad which permits an an-

37 1942 1988 The American Physical Society

Page 2: target

37 ONE-NUCLEON STRIPPING REACTIONS TO DISCRETE. . . 1943

gular binning of 0.4 in the angular distributions. Theabsolute values for all cross sections were easily obtaineddue to the fact that the measured ' C elastic cross sectionobeys the Rutherford law at forward angles.

III. RKSUI.TS AND DISCUSSION

First, we shall present and discuss the results of theone-nucleon stripping reactions populating the low lyingsingle particle states which have well-known spin assign-ments. Secondly, we shall present the results of thetransfer data populating states at higher excitation ener-

gy for which high spin single particle configurations havebeen rather hypothetically assigned. Then finally, weshall present a general discussion concerning the EFR-DWBA predictions of cross section absolute values forone-nucleon stripping reactions.

A. One-nucleon stripping reactions populatingthe low lying single particle states

In Fig. 1 is presented the energy spectrum of thePb(' C, "B) Bi one-proton stripping reaction mea-

sured at 480 MeV ' C incident energy along with the en-

ergy spectrum of the Pb(' 0, ' N) Bi one-protonstripping reaction measured at 793 MeV ' 0 incident en-

ergy. ' The relative intensities of the populations of thevarious single-particle states can be explained with thetwo selection rules previously discussed in the Introduc-tion. For the (' C, "B}reaction the strongest peak is the1.608 MeV li ", —+ favored by the two selection rules (i)

high final angular momenta, l =6, and (ii) no spin fliptransition: 1f+—,', (li "+—) final spin in Bi residual nu-

cleus for a I, +—,'(Ip —', ) initial spin in the projectile. On

the other hand, for the (' 0, "N) reaction (initial stateIp —,', 1;——,

' in the projectile), the transition to the 1.608MeV li —", + which corresponds to a spin flip process is in-

hibited despite the large orbital angular momentum in-volved in the transfer process. For the (' 0, ' N} reac-tion, the g.s. lh —', , I =5 transition is favored by the twoselection rules and is thus the strongest peak for thisstripping reaction, but in case of the (' C, "B) reactioninvolving a spin flip transition, we observe a small peakfor the g.s. yield: the transition is inhibited. Other in-teresting lines are the 2f—,

' and 2f—,' states both 1=3

transitions. It is then only the second selection rule con-cerning spin flip transitions which can explain thedifferences in intensities between these two levels in the(' C, "B) and (' 0, ' N) one proton stripping reactions.For the (' 0, ' N) reaction, the no spin flip transition cor-

2400

1500—

1000—

Pb (' C "8) Bi

E+ = 480MeV

3.8 g e)~g 4 2

2000—

1600—

1200—

204pb {12C 11C~ 209pb

E+ = 480HeV

5 4'~e g5 8'

500— 800—

600—

400—

200—

f I

2OIPb {14O 15Nj 2098j

E~ = 793MeV

3' 8+&4 754

)4JZCo +

Eh4m~ o

400—

LJ

200—

20$Pb (lhP sP} 20%Pb

E~ = 793NeV

3 25o~e)~~4 75o

OlE

/Pl

J,J11~lj

01075

A.1100 1125 1150 1175 1200 1225

CHANNEL

100—

1150 1175 1200

CHANNEL

1225 1250

FIG. 1. Energy spectra for the one-proton stripping reactionsinduced by ' 0 and ' C beams at 793 and 480 MeV incident en-

ergies, respectively. Only high spin single-particle states arepopulated strongly. The energy resolution is about 200 keVFWHM.

FIG. 2. Energy spectra for the one-neutron stripping reac-tions induced by ' 0 and ' C beams at 793 and 480 MeV in-

cident energies, respectively. Only high spin single-particlestates are populated strongly. The energy resolution is about200 keV FWHM.

Page 3: target

1944 M. C. MERMAZ et al. 37

responds to the 2.822 MeV 2f—,' state which has a

stronger counting yield than the 2f—,'level, see bottomof Fig. 1. On the other hand, the no spin flip transitionfor the (' C, "B) reaction corresponds to the 0.896 MeV2f ,'st—ate which has a stronger counting yield than the2f—', level, see top of Fig. l. For both one-proton strip-

ping reactions let us note that the orbital angular momen-tum mismatch between the entrance and exit channel is8A for the grazing waves. This value of 8A is obtained byinspection of the optical model S matrix elements of theentrance and exit channel: S« ——0.50. See later on, theelastic scattering and DWBA analysis. Other levels arepopulated in the (' C, "B) reaction spectrum and will bediscussed later on. In case of the (' 0, ' N) reactionsthese additional lines are obscured by the excitation ofthe ejectile in its 1p—, single hole-state located at 6.324MeV, see Refs. 4, 5, and 2.

In Fig. 2 are presented the one-neutron stripping reac-tion spectra induced by ' C and ' 0 projectile, respective-ly, on a Pb target. The interpretation of these data fol-low the previous discussion. The strongest transitions forboth reactions involve large angular momenta and nospin flip: they are the 1.423 MeV 1j—", level, 1=7, forthe (' C, "C) reaction and the 0.779 MeV li —", + level forthe (' 0, ' 0) reaction. '-' Let us note that the orbital an-gular momenta mismatch for the grazing waves is 10% forboth stripping reactions. The populations of the 2g—', +

and 2g—,'+ states, both I =4, are governed in the two ener-

gy spectra only by the no spin flip selection rule; andtheir relative strengths are inverted in the two reactions.Other lines are also populated at higher excitation energyin the (' C, "C) reaction and will be discussed later on.These lines are obscured in the (' 0, ' 0) reaction by theexcitation of the ' 0 ejectile on its 1p—,

' single hole statelocated at 6.176 MeV, see Refs. 4, 5, and 2.

In order to obtain absolute values for the stripping re-action cross sections and in order to perform a full EFR-DWBA calculation, the ' C elastic scattering angular dis-tribution has been measured. A Fresnel pattern is ob-served and has been analyzed in the framework of the op-tical model using in all our calculations a volumeWoods-Saxon geometry for the real and imaginary partof the potential. A typical result of a best fit procedure ispresented in Fig. 3 ~ It was obtained with the codepToLEMY (Ref. 9) which has no relativistic correction forelastic scattering and direct transfer reaction calcula-tions. The family given in Fig. 3 corresponds to strongabsorption and many other families can be deduced fromthe Igo ambiguity. ' This present family of Fig. 3 is aliketo the one used to analyze the stripping reactions inducedby the 793 MeV ' 0 beam bombarding a Pb target. Itis worthwhile to note that this 50 MeV deep potential hasits parameter values, in best agreement with the theoreti-cal predictions of the energy density formalism used withthe sudden approximation. "' Results of full EFR-DWBA calculations for the one-nucleon stripping reac-tion, using deeper volume Woods-Saxon potentials withor without equal geometry for the real and imaginaryparts, will be also presented later on in the section dis-cussing the absolute cross section values; see Tables V

Pb ( C Lj

E)~— 080 MeV

C

b

CD

b

01=

001 =

PTOLE

V = W = 50.0oc = roc = r

ao = ai = 0.792-099

I I I I I I I I I I I I

4 6 8 10 12 14

ec.m ~4egj

FIG. 3. Elastic scattering angular distribution of the 480MeV ' C beam on the 'Pb target along with the optical modelparameters of volume Woods-Saxon family B3 and the averagechi-square value per point.

and VI of Sec. III C.Figure 4 presents the results of the full EFR-DWBA

calculations using the optical model parameter family ofFig. 3 which best fit the elastic scattering data, and usingalso the form factor parameters for the projectile and theheavy residual nucleus coming from Table III of Ref. 2.The spectroscopic factors were extracted using the usualformula:

2olpb ~12t 11B~ 2O9g

E& = 480 NeV

100—4

4 . , 1.608 MeV 1i 13/2'

C'

~ 0.896 M

10—2.822 M

rrr 04

a

4 .s. 1h 9/2

PTOLEMY

V=W=50.

a, = a; = 0.7915fmI I I I

3 5

8, (deg)

FIG. 4. Angular distributions for the Pb( ' C, "B) Bione-proton stripping reaction. The solid lines are the results ofEFR-DWBA calculations; see text and the spectroscopic factorsof Table I.

Page 4: target

37 ONE-NUCLEON STRIPPING REACTIONS TO DISCRETE. . . 1945

TABLE I. One-proton spectroscopic factors for the Bi final nucleus.

State

2

2f7—

„»+'2

2f 5—

(MeV)

g.s.0.8961.608

(16O 15N)

793 MeV

0.75

0.670.70

0.74

(12C 11B)

480 MeV

0.48

0.660.70

0.80b

(a, t)80 MeV

0.75

0.71

0.70

0.54

Theory'

0.950.85

0.70

'All the spectroscopic factors are normalized to the 1.608 MeV li —",+ state theoretical value, Ref. 15,

this letter value is underlined in the table. The 1.608 MeV li —"+ level is the most strongly populated

state in the (' C, "B)reaction.The contribution of the 2.601 MeV li—'+ level has been subtracted assuming a spectroscopic factor of

0.06 for this state, Ref. 14.

da, „~,(8)=NS;SfdcrDwnA(~)

where S; is the one-nucleon spectroscopic factor of theprojectile-ejectile system and equals to 4 for ' C nucleus:1p—', orbit completely filled; Sf is the spectroscopic fac-tor for the heavy residual nucleus; the cross sectiond0DwaA(8) is provided by the code PTOLEMY (Ref. 9) andN is an overall normalization factor which is equal to 1 ifthe EFR-DWBA model is perfectly suitable to analyzesuch a direct stripping reaction assuming a one-step pro-cess. As a matter of fact, we can say that final state spec-troscopic factors are known only in relative value. At theend of this paper we shall discuss the problem of normali-zation factor N whose value depends on the form factorparameters and on the optical model parameters.

It is worthwhile to note that the present geometry ofthe form factor parameters best fits the single particlestate energies either of Pb or Bi see Ref. 3. It hasalso been checked that the code SATURN-MARS-I (Ref. 13)provided identical results as the code PTOLEMY (Ref. 9).

In Table I are presented the spectroscopic factors forthe first single particle states of Bi. In Fig. 1 it can benoticed that the 2f—', line located at 2.822 MeV excita-tion energy is broad. This is due to a contribution fromthe 2.601 MeV li —",

+ state favored by the tan selectionrules. The spectroscopic factor of this 1i —",

+ state is 0.06(Ref. 14). In order to extract the spectroscopic factor ofthe 2f—,'state, this small contribution was theoreticallycalculated and then subtracted. These spectroscopic fac-tors are similar to those obtained previously in the(' 0, ' N) reaction and in the (a, t) reaction, ' both per-formed on Pb target. For the (' C, "B) reaction, theg.s. spectroscopic factor seems to be too weak. In Table Iwe have quoted the results of a quasiparticle calculation'which agree rather well with our results. Thus it can beconcluded that EFR-DWBA calculations reproduce fair-ly well the relative intensities of the Pb(' C, "B) Bione-proton stripping reaction. However, the EFR-DWBA fits of Fig. 4 are rather poor at backward angles,inducing an uncertainty of about 10 to 20% on the spec-troscopic factor values.

Figure 5 presents the results of the EFR-DWBA calcu-lations for the angular distributions of the

Pb(' C, "C) Pb one-neutron stripping reactions mea-sured at 480 MeV ' C incident energy. As discussed pre-viously, the form factor parameters come from Table IIIof Ref. 2 and best fit the single particle state excitationenergies. The optical model parameters are those inset inFig. 3, family 83, which best fit the ' C elastic scatteringdata. The agreement between the experimental pointsand the calculated angular distributions is strikingly goodfor this one-neutron stripping reaction. Table II gives thespectroscopic factors extracted from this analysis. They

I I

2oapb(i2C n&) 2ovpb

Eg& = 480MeV

100:&~ ' o-&~-'~~w:1.423MeV (1j 15/2 )

C:

~P 010 = g.s. {2g 9/2')

3k

10=

0.779MeV {1i 11/2 )

wo

2.491MeV (2g 7/2')

V =

r 0

a, =

PTOLEMY

W = 50.0NeVr = r = 1.0821fm

a; =0.7915fmI I I

5 7

8, (deg )

FIG. 5. Angular distributions for the Pb("C, "C) Pb oneneutron stripping reaction. The solid lines are the results of theEFR-DWBA calculations; see text and spectroscopic factors ofTable II.

Page 5: target

1946 M. C. MERMAZ et al. 37

TABLE II. One-neutron spectroscopic factors for the Pb final nucleus.

State

2g 2

1 —"+

(Mevi

g.s.0.7791.423

(16O 15O)

793 MeV

0.890.72

0.62

(12C 11C)

480 MeV

0.800.500.62b

(a, 'He)183 MeV

0.76

1.030.62

Theory'

0.890.960.62

2g7 + 2.491 0.79 0.92'

'All spectroscopic factors are normalized to the 1.423 MeV 1j'~' state theoretical value, Ref. 15, this

latter value is underlined in the table. The 1.423 MeV 1j—" level is the most strongly populated state

in the (' C, "C) reaction.For the 1.423 MeV 1j—", , it has been checked that the EFR-DWBA cross section of the unresolved

1.567 MeV 3d 2+ state is negligible due to the large momentum mismatch.

'For the 2g —,'+, it has been checked that the EFR-DWBA cross section of the unresolved 2.537 MeV

3d—'+ state is negligible due to the large momentum mismatch and to the violation of the no spin-flip2

selection rule.

agree rather well with the previous data of the (' 0, ' 0)reaction and also with the quasiparticle calculations, ' ex-ception made for the 0.779 MeV li —", level. Othertheoretical spectroscopic factors of single particle stateseither for neutron or proton direct transfer reactions canbe found in the review article of Mahaux et al. ' andreferences therein.

2000'

1600-

1200-

800-

201Pb ~$2C 11C~ 209Pb

E&= 480HeV

74 +el b&82

B. One-nucleon stripping reactions populatingthe higher excited states

Now we shall present a tentative analysis of the strip-ping reactions populating the higher excited levels of the

Bi and Pb residual nuclei. For these levels the spinassignment is rather hypothetical and comes from Refs.17 and 18. The main interest of these heavy ion reactionsat high incident energy is that they populate stronglyonly high spin states. On the other hand our energy reso-lution is only 200 keV F%HM. Several excited levels canbe seen in the spectrum of Pb (Fig. 6): possible 1j—",

and 1k —", + candidates from the work of Massolo et al. '

Such levels of / =7 and l =8, respectively, are stronglyfavored by the two previous selection rules in the(' C, "C) reaction. These levels can be followed at all theangles. They are the 3.02 MeV 1j—", level, the 3.59 MeV

1j—", and 3.73 MeV 1j—", doublet, and the 3.96 MeV1k —", + and 4.22 MeV 1k —", + doublet. Above this groupof levels, broad structures can be observed on the variousenergy spectra around an excitation energy of 10 MeVwhich is the energy position of giant quadrupole reso-nance, see Ref. 19.

Figure 7 presents the angular distribution of the excit-ed levels of Pb heavy residual nucleus. The values ofthe experimental points were obtained by a best fit pro-cedure of the energy spectrum lines without any back-ground. The agreement in shape of the angular distribu-tion is rather reasonable. The corresponding spectro-scopic factors are listed in Table III. They agree more orless with the ones obtained by the (a, He) experiment, '

exception made of the hypothetical 1k—", + doublet locat-ed at 4.1 MeV excitation energy. This doublet is un-

400-8 -—-e

2000-

1600—

1200—

800-

400~ -- --- --- -- ~~M~

I I I iI

2000-C)LJ

5 8 &Stat &6 61600—

1200- XNg Vw aE

800—

IA

~ fVrv

~ N

400-

2000—

1600—

1200—

5' 8),b4;5.8

10MeV

800-

400-

I I

400 500 600 700 800 900

CHANNEL

FIG. 6. Energy spectra of the pb( "C,"C)"'pb oneneutron stripping reaction at several laboratory angles present-ed in order to follow the weakly excited states of high spin lo-cated at high excitation energies.

Page 6: target

37 ONE-NUCLEON STRIPPING REACTIONS TO DISCRETE. . . 1947

C:

0

100:

10 =

2ospb(12( 11p)209pb

E g~ = 480Me Y

PTOLEMYV = W = 50.0MeV

r, = r„= r, = 1.0821fm

a, = a, = 0.7915fm

3.02MeV (1j 15/2 )

3.6MeV (1j 15/2 )

confidence about this procedure of spectroscopic-factorextraction. It is also worthwhile to note that Hartree-Fock calculations predict a lk —",

+ level around 6 MeVexcitation energy.

Figure 8 presents the one-proton stripping reactionspectra measured at several angles. Several states athigher excitation energy can be followed at each angle be-tween the 3.87 MeV li —",

+ state and the 5.44 MeV 1J,'li —", + unresolved multiplet. Furthermore, as in the one-

208Pbl12[ 11@209B~

Empt- = 480Hev

7 0'&8 &8.2'2—

10—4.06MeV (1k 17/2')

t I

5

B,m («g) 6.64&8 &7.44lab

FIG. 7. Angular distributions for the 'Pb(' C, "C) Pbone-neutron stripping reaction. The solid lines are the results ofthe EFR-DWBA calculations. See text and spectroscopic fac-tors of Table III.

bound and the EFR-DWBA analysis has been performedin the following way. First of all, the experimental Qvalue is input in the FTOLEMY (Ref. 9) code for the dis-torted wave calculations: the usual procedure. However,the 1k —", + wave function is arbitrarily bound by —0. 10MeV. It has been checked that a binding energy of—0.50 MeV increases the spectroscopic factor values byonly 8%. It is worthwhile to note that the lk —",

+ doubletexcitation energy is very near to the Pb neutron bind-ing energy: 3.9364 Me V. So we may have some

rn

X

L/l 0 t

o

0 i

5 8'&8 «6 6'lab

CV

Vl ~V

4I

EfV

State {MeV)

(12C 11C)

480 MeV(a, 'He)

183 MeV

TABLE III. One-neutron spectroscopic factors or sums forthe Pb final nucleus. All spectroscopic factors of Pb arenormalized on the 1.423 MeV 1j'2' theoretical value of Table

II; the spin assignments between parentheses are rather hy-pothetical and come from Ref. 18.

8 — 54 8 ~584lab bc 4 t

PV

I:EECh N gg

3.023.59

0.085

0.065

0.057

0.076

0 1

400 500l I

600 700

CHANNEL

800 900

(1k—"+)2

3.73

3.96

4.220.13 0.064

FIG. 8. Energy spectra pf the Pb(' C, "B) Bi one-protonstripping reaction at several laboratory angles presented in or-der to follow the weakly excited states of high spins located athigh excitation energies.

Page 7: target

1948 M. C. MERMAZ et al. 37

neutron stripping reaction, a structure at an excitationenergy of about 10 MeV can be seen for which onlyspeculation can be made about its origin: excitation in atwo-step process of single-particle states coupled to thetarget giant quadrupole resonance. The cross-sectionvalues were extracted from these energy spectra using abest fit procedure with a smooth empirical backgroundgoing through the deepest valley of the energy spectra.This procedure will give rise to a large uncertainty in thespectroscopic factor values. Figure 9 presents EFR-DWBA fits of the angular distributions of these excitedlevels which are all unbound, the proton binding energyis 3.7980 MeV, and in these calculations the wave func-tions have been arbitrarily bound by —0. 10 MeV. Ex-ception made of the 4.26 MeV 1j—", state, the fits arerather acceptable and the corresponding spectroscopicfactors or their sums are given in Table IV. The li —",

+

states and all the fragmented 1j—", states are stronglyfavored by the two selection rules. On the other hand,the populations of the li —", + states are inhibited due totheir spin Aip transition. Exception made of the higherexcited multiplet, the agreement of the spectroscopic fac-tors between the (' C, "B) and (a, t) experiments' is al-most satisfactory.

State

1~ 13 +'2

( 1j15 —)

( 1j15 —)

(1j—", )

(MeV)

3.835

4.17

4.27

4.88

4.995.27

5.38

5.47

5.58

(lzC, &iB)

480 MeV

0.017

0.063

0.021

0.018

(a, t)80 MeV

0.028

0.099

0.047

0.16

C. The EFR-DWBA predictions ofcross section absolute values

TABLE IV. One-proton spectroscopic factors or sums forthe Bi final nucleus. All spectroscopic factors of ' Bi arenormalized on the 1.608 MeV li'z theoretical value of Table I.The spin assignments between parentheses are rather hypotheti-cal and come from Ref. 17.

102

208pb(12' 11B)2098

E» = 480 NeV12t-

10:.26NeV (1j15/2 )

C:4.99NeV (1j

4MeV (1j15/2 )

3.873 NeV 1i 13/2

10 'I I

5

8, (deg)

FIG. 9. Angular distribution for the Pb(' C, "B) Bi one-proton stripping reaction. The solid lines are the results of theEFR-DWBA calculations; see text and spectroscopic factors ofTable IV.

We are going to discuss now the problem of the abso-lute values for the cross sections at high incident ener-gies. Although the EFR-DWBA calculations predictcorrectly the absolute cross-section values for the one-nucleon stripping reactions induced by the 480 MeV ' Cbeam, it has turned out that for the one-nucleon strippingreactions induced by the 793 MeV ' 0 beam the absolutecross-section values are overpredicted by a factor of5 —10, see Refs. 4 and 5.

In order to study the stability of the cross-sectionvalues with respect to the variation of the optical modelparameters for the ' C beam experiments, we have tried adeeper volume Woods-Saxon family of potentials, namelyV = W =200 MeV, which also best fits the elastic scatter-ing data. Thus potential is drawn in Fig. 10 along withthe V= 8'=50 MeV family. We can see that both fami-lies exhibit the same tails. This fact is just the signatureof the continuous Igo ambiguity. ' This newV= 8'=200 MeV family reproduces perfectly well thedata and provides the stripping cross sections with al-most the same absolute values; in other words, the samenormalization coefficient X, see formula (l). These twofamilies (the 50 MeV and 200 MeV), have equal geometryfor the real and imaginary part. To check the sensibilityto this feature we have also performed calculations withfamilies having a different geometry for the real andimaginary part. They were obtained by increasing or de-creasing the radius parameter of the imaginary part by30%, 20%, or 10% and then searching with the automat-ic code pTQLEMY (Ref. 9) for the best elastic scattering fit

by varying the imaginary depth and imaginary difFusivityand keeping the same real part geometry of the V=200MeV or of the V =50 MeV family A and B, respectively.In Table V are listed the various potentials with their cor-responding 7 values for elastic scattering and with the

Page 8: target

37 ONE-NUCLEON STRIPPING REACTIONS TO DISCRETE. . . 1949

50)K

0—

12I

u~, zospb

Eac = 080NeV

181

R(fm)

-50 IIII-100— I

lI

I-150— l/

I-200 ———

V=V r)(MeV) (fe) tfm)

-50.0 1.0S21 0.7915

-200.0 0.9047 0.8560

FIG. 10. Real and imaginary part of the volume Woods-Saxon family A 3 and B3 used for the various EFR-DWBA cal-

culations. Both potentials best fit the ' C elastic scattering dataon 'Pb target.

normalization coefficient N values. These coefficients Nwere determined from the g.s. transitions using the corre-sponding experimental spectroscopic factors of Bi and

Pb final nuclei, respectively, see Tables I and II. Theimaginary parts of the various potentials are plotted inFigs. 11 and 12. The following comments can be made.All the optical potentials which have the same tails pro-duce both excellent EFR-DWBA fits for the one-nucleonstripping angular distributions and reasonable normaliza-tion coefficients N. This is the case for all the families 3( A I —A 5) and for the families 83, B4, and 85. FamiliesB1 and B2 are dubious, producing very poor EFR-DWBA fits for the one-nucleon stripping reaction, and,furthermore, their elastic scattering g values are notvery good. From Fig. 12 we can see that their tails arenot correct since their imaginary wells are not deepenough.

The same systematic analysis was also performed forthe one-nucleon stripping reactions induced by the 793MeV ' 0 beam on a Pb target. Figure 13 shows a typi-cal result of an EFR-DWBA analysis obtained for the(' 0, ' N) one-proton stripping reaction, with theV=@'=200 MeV family C3. The agreement in shapefor the angular distributions is strikingly good and thecorresponding spectroscopic factors are similar to thosequoted in Table I. Let us also note that the (

' 0, ' 0) oneneutron stripping reaction on Pb provides similar spec-troscopic factors as those of (

' C, "C) reaction, see Ref.5. Table VI presents for the one-neutron and the oneproton stripping reactions the normalization coefficientsN of the EFR-DWBA analyses performed with potentialssimilar to those used for the ' C beam and listed alreadyin Table V. As previously, these coefficients N are deter-mined from the g.s. transitions using the correspondingspectroscopic factors of Ref. 5 for Bi and Pb finalnuclei. All the C families (200 MeV deep potential forthe real part) produce similar EFR-DWBA fits for thetransfer data and a similar coefficient of normalization Nof the order of 0.15. The same results are reached for thefamilies D3, D4, and D5, having a real potential 50 MeVdeep. Nevertheless, for the shallow imaginary well, fami-lies D1 and D2 fail to reproduce the experimental data inshape and in absolute value.

All the EFR-DWBA curves obtained with the opticalmodel parameters which reproduce the entrance channelelastic scattering are very similar and produce normaliza-tion factors obtained in the same consistent way. Howev-er, the DWBA fits are not very good in case of (' C, "B)one proton stripping reactions exception mode of the g.s.transition. It is generally considered that spectroscopicfactors and normalization coefficients have to be extract-ed by fitting the experimental angular distributions at for-ward angles where the theoretical curves are less depen-dent of the optical model parameters. Normalization fac-tors taking more into account the backward angle mea-surements will decrease the normalization factor by 20%especially for the excited levels of Bi. It has beenshown by Peng et al. , Ref. 20, that in case of Fresnel elas-tic scattering pattern in the entrance and exit channels,

TABLE V. Coefficient N of normalization for the one-nucleon stripping reactions for the system' C+ Pb at 480 MeV incident energy. Real part of the volume Woods-Saxon families A: V=200.0MeV, ro ——ro ——0.9047 fm, a =0.8360 fm. Real part of the volume Woods-Saxon families B: V=50.0

C

MeV, ro =ro ——1.0821 fm, a =0.7915 fm.

Family

A1A2A3A4A5B1B2B3B4B5

8(MeV)

25.42.4

200.473.

1111.48.2

10.250.

134.2378.8

(fm)

1.1761.0850.9040.8140.7231.4061.2981.0820.9730.865

a;(fm)

0.8120.8190.8560.8500.8530.5740.6580.7910.8110.822

1.931 ~ 121.161.291.255.021.530.991 ~ 161.29

N(' C ''B)

0.970.640.740.730.740.280.240.790.830.92

N( i~C, l lC)

1.110.830.870.850.861.320.740.980.941.00

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1950 M. C. MERMAZ et al. 37

0—

12I

12' 208 pb

Eg~ — 480NeV

18I

-60—

-120—

-180—

-240—

/~

/j

r;(MeV) (fNI) (fm)

-25.0 1.1760 0.8125

-42.4 1.0856 0.8190

-200.0 0.9047 0.8560

-473.0 0.8142 0.8508

-1111.4 0.7238 0.8532

FIG. 11. Volume Woods-Saxon imaginary part of the opticalmodel potential used in the EFR-DWBA calculations. The realparts of all these families have their parameters equal to thoseof family A3. All best fit the elastic scattering data. It hasturned out that all these potentials produce the same results forthe elastic scattering cross sections and for the one-nucleon

stripping cross sections since they have the very same tails.

The normalization coefficients, N, can be slightly de-creased by increasing the radii of the form factor. Forthe bound state wave function of the heavy residualpartners the radius parameters are already large 1.28 and1.25 fm for the Bi and Pb, respectively, but for the' C projectile an increase of the radius parameter from1.20 fm to 1.25 fm produces a decrease of the normaliza-tion coefficient of 10%. Furthermore, the value of thenormalization coefficient N, depends, according to formu-la (1), on the value of the entrance channel spectroscopicfactor. We have taken so far crude shell model estimates:4 and 2, respectively, for the ' C and ' 0 projectiles.However, from the ' C( He, a)"C pick-up reaction and' C(p, d)"C pick-up reaction the spectroscopic factorsare 3.06 and 2.5, respectively. ' These values will in-crease the normalization coefficient N by 24% and 38%%uo,

respectively. For the ' 0 projectile, we are dealing with adouble magic nuclei. Thus a value of 2 for the probablycompletely filled 1p—,

' subshell is a very reasonable as-

sumption which is confirmed by the experimental spec-troscopic factor values extracted from the one nucleonpick-up reactions induced by deuteron beam on 0 tar-16

get nucleus, see Ref. 22.To summarize the results about one-nucleon stripping

reactions induced either by a C beam or a 0 beam, we12 16

10'

the optical model parameters can be very alike for bothchannels; see Figs. 3 and 4 of Ref. 21. Due to this factand in order to avoid any arbitrariness, we have not triedto improve the EFR-DWBA fits in case of (' C, "B)oneproton stripping reactions, by using different opticalmodel parameters for the entrance and exit channels.

R(fm)

C

lh

J36

10

Pb( 60 N) 8

E16 - 793 MeV0

g.s. 1h 9/2a

v(I t)MeV 1i 13/2

20—X:

0—

)2

12t. 208pb

EL- = 480NeV

18

1O'

2.822 MeV 2f 5/24

-20—

-60—

-80

W

(Hev)r, al

(fNl) (fm)

-S.2 1.4067 0.5746—-10.2 1.2985 0.6586

-50.0 1.0821 0.7915

-134.2 0.9739 0.8115

-378.S 0.8657 0.8224

I

100

Y 2f 7/2

PTOLEMY

V = W = 200.0 MeV

rp-

r0— r. = 0.8985 fm

0 Oc

eo = a = 0.8575 feI

I I I I

4 5 68 (det) )

C.Q.

FIG. 12. Volume Woods-Saxon imaginary part of the opticalpotential used in the EFR-DWBA calculations. Families Bland B2 do not reproduce successfully the elastic scattering dataand the transfer data, while the other families do.

FIG. 13. Angular distributions for the ' Pb(' 0, "N) Bione-proton stripping reaction. The solid lines are the results ofthe EFR-DWBA calculation; see text. The corresponding nor-malization coefficient, N, is given in Table VI, family C3.

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37 ONE-NUCLEON STRIPPING REACTIONS TO DISCRETE. . . 1951

TABLE VI. Same as Table V for the system ' 0+ Pb at 793 MeV incident energy. Real part ofthe volume Woods-Saxon families C: V=200.0 MeV, ro ——ro ——0.8983 fm, a =0.8575 fm. Real part of

C

the volume Woods-Saxon families D: V=50.0 MeV, ro=ro ——1.0970 fm, a =0.7260 fm.C

Family

C1C2C3C4C5D1D2D3D4D5

W(MeV)

24.942.3

200.0454.4

1023.95.108.98

50.0113.6358.6

(fm)

1.1681.0780.8980.8080.7181.4261.3161.0960.9870.877

a,(fm)

0.7750.8050.8570.8440.8530.2530.6020.7260.7480.761

3.042.041.651.601.622.673.981.701.611.60

N(' 0, ' N)

0.170.130.140.120.120.010.030.180.120.13

N( 16P 15P )

0.150.110.150.110.110.030.110.170.100.11

can say that the normalization coefficients are of the or-der of 1 for the 480 MeV ' C projectile and of the orderof 0.10-0.20 for the 793 MeV ' 0 projectile. Let us notethat the normalization coefficient was already 0.35 at 312MeV ' 0 incident energy for this latter projectile, seeRef. 2. On the other hand, one neutron pick-up reactionsand one neutron stripping reactions induced by several' C beams in the vicinity of the Coulomb barrier on Pbtarget have provided EFR-DWBA normalization factorsN of the order of unity, see Ref. 23.

This difFerence does not come from the theoretical cal-culations but is a true experimental fact. For instance, inthe one nucleon stripping reaction induced by a ' 0 pro-jectile, the highest cross sections are 5.5 mb/sr for thelh —', g.s. of Bi and 6 mb/sr for the li —", + state of Pbat the same 4.2 c.m. angle, respectively, while in case of' C projectile the highest cross sections are 55 mb/sr forthe li ", + sta—te of Bi and 72 mb/sr for the 1j—", state of

Pb: basically a factor of 10 in the experimental crosssection values for the two different projectiles. Thus oneproton and one neutron stripping reactions appear to beinhibited at high incident energy for ' 0 beams.

These results about the ' 0 beams are rather puzzlingsince for the one proton pick-up and one-neutron strip-ping reactions induced by the ' 0 projectile bombardinga Si target at 352 MeV incident energy the normaliza-tion factors are also equal to unity for strong absorptionpotential. Furthermore, single-nucleon transfer reac-tions induced by 376 MeV ' 0 beam on a Pb target

and by Si beams of 6 and 8 MeV/nucleon incident ener-

gy, respectively, are also correctly predicted by EFR-DWBA calculations.

IV. CONCLUSION

At very high incident energy it has turned out that therelative intensities for the population of single-particlestates are governed by two selection rules contained ei-ther in the EFR-DWBA or in the semiclassical model.The strongest excited levels are single-particle high-spinstates populated without spin Nip. Reliable spectroscopicfactors can be extracted at high incident energy as well asat low energy. Absolute values of cross sections arecorrectly predicted by the EFR-DWBA using strong ab-sorption optical model potentials, where both elasticscattering cross sections and transfer reaction data arewell fitted. However, in the case of ' 0 beam the EFR-DWBA calculations fail completely to reproduce thecross sections in terms of absolute values; and this is arather puzzling problem.

ACKNOWLEDGMENTS

It is a pleasure to thank Professor C. A. Whitten, Jr.from the University of California, Los Angeles for carefulreading of the manuscript and enlightening discussions.Sincere thanks are also due to Mrs. J. Sauret and theoperating staff of the GANIL cyclotrons for the excellentquality of the 480 MeV ' C beam.

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